X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron

Isabelle Llorens; Pier Lorenzo Solari; Bruno Sitaud; René Bes; Sebastiano Cammelli; Hervé Hermange; Guillaume Othmane; Sami Safi; Philippe Moisy; Sandrine Wahu; Carole Bresson; Michel L. Schlegel; Denis Menut; Jean Luc Bechade; Philippe Martin; Jean Louis Hazemann; Olivier Proux; Christophe Den Auwer

doi:10.1515/ract-2013-2241

X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron

Isabelle Llorens
, Pier Lorenzo Solari^*
, Bruno Sitaud
, René Bes
, Sebastiano Cammelli
, Hervé Hermange
, Guillaume Othmane
, Sami Safi
, Philippe Moisy
, Sandrine Wahu
, Carole Bresson
, Michel L. Schlegel
, Denis Menut
, Jean Luc Bechade
, Philippe Martin
, Jean Louis Hazemann
, Olivier Proux
, Christophe Den Auwer

^*Tämän työn vastaava kirjoittaja

Ei julkaistu Aalto-yliopiston affiliaatiolla

CNRS- Université Paris-Saclay
CEA, Grenoble
UMR7095
Université Paris-Sud
CEA Saclay, CEA, DSM Irfu SPP
Néel Institute – CNRS, Grenoble Alpes University
Université Joseph Fourier Grenoble I
Université Côte d'Azur

Tutkimustuotos: Lehtiartikkeli › Article › Scientific › vertaisarvioitu

54 Sitaatiot (Scopus)

Abstrakti

The MARS beamline at the SOLEIL synchrotron is dedicated to the characterization of radioactive material samples. One great advantage of the beamline is the possibility to characterize about 380 radionuclides by different X-ray techniques in the same place. This facility is unique in Europe. A wide energy range from around 3.5keV to 36keV K-edges from K to Cs, and L3 edges from Cd to Am and beyond can be used. The MARS beamline is optimized for X-ray absorption spectroscopy techniques (XANES/EXAFS), powder diffraction (XRD) but x-ray fluorescence (XRF) analysis, High Energy Resolution Fluorescence Detected -XAS (HERFD-XAS), X-ray Emission (XES) and μ-XAS/XRD are also possible. A description of the beamline as well as its performances are given in a first part. Then some scientific examples of XAS studies from users are presented which cover a wide variety of topics in radiochemistry and nuclear materials.

Alkuperäiskieli	Englanti
Sivut	957-972
Sivumäärä	16
Julkaisu	Radiochimica Acta
Vuosikerta	102
Numero	11
DOI - pysyväislinkit	https://doi.org/10.1515/ract-2013-2241
Tila	Julkaistu - 1 tammik. 2014
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

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10.1515/ract-2013-2241

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Llorens, I., Solari, P. L., Sitaud, B., Bes, R., Cammelli, S., Hermange, H., Othmane, G., Safi, S., Moisy, P., Wahu, S., Bresson, C., Schlegel, M. L., Menut, D., Bechade, J. L., Martin, P., Hazemann, J. L., Proux, O., & Den Auwer, C. (2014). X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron. Radiochimica Acta, 102(11), 957-972. https://doi.org/10.1515/ract-2013-2241

@article{0801a1016ade4b70b3a2b3e85290bd4d,

title = "X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron",

abstract = "The MARS beamline at the SOLEIL synchrotron is dedicated to the characterization of radioactive material samples. One great advantage of the beamline is the possibility to characterize about 380 radionuclides by different X-ray techniques in the same place. This facility is unique in Europe. A wide energy range from around 3.5keV to 36keV K-edges from K to Cs, and L3 edges from Cd to Am and beyond can be used. The MARS beamline is optimized for X-ray absorption spectroscopy techniques (XANES/EXAFS), powder diffraction (XRD) but x-ray fluorescence (XRF) analysis, High Energy Resolution Fluorescence Detected -XAS (HERFD-XAS), X-ray Emission (XES) and μ-XAS/XRD are also possible. A description of the beamline as well as its performances are given in a first part. Then some scientific examples of XAS studies from users are presented which cover a wide variety of topics in radiochemistry and nuclear materials.",

keywords = "HERFD-XAS, Molybdenum, Neptunium, Synchrotron, Thorium, Uranium, X-rays, XAS, Zirconium",

author = "Isabelle Llorens and Solari, \{Pier Lorenzo\} and Bruno Sitaud and Ren{\'e} Bes and Sebastiano Cammelli and Herv{\'e} Hermange and Guillaume Othmane and Sami Safi and Philippe Moisy and Sandrine Wahu and Carole Bresson and Schlegel, \{Michel L.\} and Denis Menut and Bechade, \{Jean Luc\} and Philippe Martin and Hazemann, \{Jean Louis\} and Olivier Proux and \{Den Auwer\}, Christophe",

year = "2014",

month = jan,

day = "1",

doi = "10.1515/ract-2013-2241",

language = "English",

volume = "102",

pages = "957--972",

journal = "Radiochimica Acta",

issn = "0033-8230",

publisher = "De Gruyter",

number = "11",

}

Llorens, I, Solari, PL, Sitaud, B, Bes, R, Cammelli, S, Hermange, H, Othmane, G, Safi, S, Moisy, P, Wahu, S, Bresson, C, Schlegel, ML, Menut, D, Bechade, JL, Martin, P, Hazemann, JL, Proux, O & Den Auwer, C 2014, 'X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron', Radiochimica Acta, Vuosikerta 102, Nro 11, Sivut 957-972. https://doi.org/10.1515/ract-2013-2241

TY - JOUR

T1 - X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron

AU - Llorens, Isabelle

AU - Solari, Pier Lorenzo

AU - Sitaud, Bruno

AU - Bes, René

AU - Cammelli, Sebastiano

AU - Hermange, Hervé

AU - Othmane, Guillaume

AU - Safi, Sami

AU - Moisy, Philippe

AU - Wahu, Sandrine

AU - Bresson, Carole

AU - Schlegel, Michel L.

AU - Menut, Denis

AU - Bechade, Jean Luc

AU - Martin, Philippe

AU - Hazemann, Jean Louis

AU - Proux, Olivier

AU - Den Auwer, Christophe

PY - 2014/1/1

Y1 - 2014/1/1

N2 - The MARS beamline at the SOLEIL synchrotron is dedicated to the characterization of radioactive material samples. One great advantage of the beamline is the possibility to characterize about 380 radionuclides by different X-ray techniques in the same place. This facility is unique in Europe. A wide energy range from around 3.5keV to 36keV K-edges from K to Cs, and L3 edges from Cd to Am and beyond can be used. The MARS beamline is optimized for X-ray absorption spectroscopy techniques (XANES/EXAFS), powder diffraction (XRD) but x-ray fluorescence (XRF) analysis, High Energy Resolution Fluorescence Detected -XAS (HERFD-XAS), X-ray Emission (XES) and μ-XAS/XRD are also possible. A description of the beamline as well as its performances are given in a first part. Then some scientific examples of XAS studies from users are presented which cover a wide variety of topics in radiochemistry and nuclear materials.

AB - The MARS beamline at the SOLEIL synchrotron is dedicated to the characterization of radioactive material samples. One great advantage of the beamline is the possibility to characterize about 380 radionuclides by different X-ray techniques in the same place. This facility is unique in Europe. A wide energy range from around 3.5keV to 36keV K-edges from K to Cs, and L3 edges from Cd to Am and beyond can be used. The MARS beamline is optimized for X-ray absorption spectroscopy techniques (XANES/EXAFS), powder diffraction (XRD) but x-ray fluorescence (XRF) analysis, High Energy Resolution Fluorescence Detected -XAS (HERFD-XAS), X-ray Emission (XES) and μ-XAS/XRD are also possible. A description of the beamline as well as its performances are given in a first part. Then some scientific examples of XAS studies from users are presented which cover a wide variety of topics in radiochemistry and nuclear materials.

KW - HERFD-XAS

KW - Molybdenum

KW - Neptunium

KW - Synchrotron

KW - Thorium

KW - Uranium

KW - X-rays

KW - XAS

KW - Zirconium

UR - https://www.scopus.com/pages/publications/84910117844

U2 - 10.1515/ract-2013-2241

DO - 10.1515/ract-2013-2241

M3 - Article

AN - SCOPUS:84910117844

SN - 0033-8230

VL - 102

SP - 957

EP - 972

JO - Radiochimica Acta

JF - Radiochimica Acta

IS - 11

ER -

X-ray absorption spectroscopy investigations on radioactive matter using MARS beamline at SOLEIL synchrotron

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