Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films

Fedor M. Kochetkov; Vladimir Neplokh; Viktoria A. Mastalieva; Sungat Mukhangali; Aleksandr A. Vorob’ev; Aleksandr V. Uvarov; Filipp E. Komissarenko; Dmitry M. Mitin; Akanksha Kapoor; Joel Eymery; Nuño Amador-Mendez; Christophe Durand; Dmitry Krasnikov; Albert G. Nasibulin; Maria Tchernycheva; Ivan S. Mukhin

doi:10.3390/nano11061503

Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films

Fedor M. Kochetkov^*
, Vladimir Neplokh
, Viktoria A. Mastalieva
, Sungat Mukhangali
, Aleksandr A. Vorob’ev
, Aleksandr V. Uvarov
, Filipp E. Komissarenko
, Dmitry M. Mitin
, Akanksha Kapoor
, Joel Eymery
, Nuño Amador-Mendez
, Christophe Durand
, Dmitry Krasnikov
, Albert G. Nasibulin
, Maria Tchernycheva
, Ivan S. Mukhin

^*Tämän työn vastaava kirjoittaja

Tutkimustuotos: Lehtiartikkeli › Article › Scientific › vertaisarvioitu

13 Sitaatiot (Scopus)

129 Lataukset (Pure)

Abstrakti

We propose and demonstrate both flexible and stretchable blue light-emitting diodes based on core/shell InGaN/GaN quantum well microwires embedded in polydimethylsiloxane membranes with strain-insensitive transparent electrodes involving single-walled carbon nanotubes. InGaN/GaN core-shell microwires were grown by metal-organic vapor phase epitaxy, encapsulated into a polydimethylsiloxane film, and then released from the growth substrate. The fabricated free-standing membrane of light-emitting diodes with contacts of single-walled carbon nanotube films can stand up to 20% stretching while maintaining efficient operation. Membrane-based LEDs show less than 15% degradation of electroluminescence intensity after 20 cycles of stretching thus opening an avenue for highly deformable inorganic devices.

Alkuperäiskieli	Englanti
Artikkeli	1503
Sivumäärä	10
Julkaisu	Nanomaterials
Vuosikerta	11
Numero	6
DOI - pysyväislinkit	https://doi.org/10.3390/nano11061503
Tila	Julkaistu - kesäk. 2021
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Rahoitus

The authors J.E., C.D. and A.K. would like to thank Jean Dussaud for his work on the MOVPE setup. V.N. would like to thank Maria Baeva for her assistance with the stretchable LED transparency measurements.J.E., C.D. and A.K. thank French National Labex GaNeX (ANR-11-LABX-0014) for MW synthesis and CL measurements. V.N. thanks the Russian Foundation for Basic Research (RFBR project no. 19-32-60040) for PDMS/MW membrane fabrication and optical measurements. I.S.M., V.N., F.M.K. thank the support from the Russian Science Foundation (grant 20-19-00256) for PDMS synthesis and electrical measurements. D.K. and A.G.N. thank Russian Foundation of Basic Research project no. 20-03-00804 for the synthesis of carbon nanotubes. F.E.K. thanks the support from the Russian Science Foundation (grant 19-79-00313) for the LED array encapsulation and membrane transfer. I.S.M., F.M.K., V.N., V.A.M., S.M., A.A.V., A.V.U., and D.A.M. thank the Ministry of Science and Higher Education of the Russian Federation (FSRM-2020-0005) for the general support. N.A. and M.T. acknowledge the financial support from the ITN Marie Curie project INDEED (grant no. 722176), by the Indo-French Centre for the Promotion of Advanced Research (IFCPAR/CEFIPRA project no. 6008-1) for MW/PDMS membrane processing and characterization. Funding: J.E., C.D. and A.K. thank French National Labex GaNeX (ANR-11-LABX-0014) for MW synthesis and CL measurements. V.N. thanks the Russian Foundation for Basic Research (RFBR project no. 19-32-60040) for PDMS/MW membrane fabrication and optical measurements. I.S.M., V.N., F.M.K. thank the support from the Russian Science Foundation (grant 20-19-00256) for PDMS synthesis and electrical measurements. D.K. and A.G.N. thank Russian Foundation of Basic Research project no. 20-03-00804 for the synthesis of carbon nanotubes. F.E.K. thanks the support from the Russian Science Foundation (grant 19-79-00313) for the LED array encapsulation and membrane transfer. I.S.M., F.M.K., V.N., V.A.M., S.M., A.A.V., A.V.U., and D.A.M. thank the Ministry of Science and Higher Education of the Russian Federation (FSRM-2020-0005) for the general support. N.A. and M.T. acknowledge the financial support from the ITN Marie Curie project INDEED (grant no. 722176), by the Indo-French Centre for the Promotion of Advanced Research (IFCPAR/CEFIPRA project no. 6008-1) for MW/PDMS membrane processing and characterization.

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CHEM_Kochetkov_et_al_Stretchable_Transparent_Light-Emitting_Diodes_2021_NanomaterialsFinal published version, 2,37 MBLisenssi: CC BY

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Kochetkov, F. M., Neplokh, V., Mastalieva, V. A., Mukhangali, S., Vorob’ev, A. A., Uvarov, A. V., Komissarenko, F. E., Mitin, D. M., Kapoor, A., Eymery, J., Amador-Mendez, N., Durand, C., Krasnikov, D., Nasibulin, A. G., Tchernycheva, M., & Mukhin, I. S. (2021). Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films. Nanomaterials, 11(6), Artikkeli 1503. https://doi.org/10.3390/nano11061503

@article{326fdf9915234ac98a12c9aee433da84,

title = "Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films",

abstract = "We propose and demonstrate both flexible and stretchable blue light-emitting diodes based on core/shell InGaN/GaN quantum well microwires embedded in polydimethylsiloxane membranes with strain-insensitive transparent electrodes involving single-walled carbon nanotubes. InGaN/GaN core-shell microwires were grown by metal-organic vapor phase epitaxy, encapsulated into a polydimethylsiloxane film, and then released from the growth substrate. The fabricated free-standing membrane of light-emitting diodes with contacts of single-walled carbon nanotube films can stand up to 20\% stretching while maintaining efficient operation. Membrane-based LEDs show less than 15\% degradation of electroluminescence intensity after 20 cycles of stretching thus opening an avenue for highly deformable inorganic devices.",

keywords = "InGaN, MOVPE, Nanowires, Single-walled carbon nanotubes, Stretchable LED",

author = "Kochetkov, \{Fedor M.\} and Vladimir Neplokh and Mastalieva, \{Viktoria A.\} and Sungat Mukhangali and Vorob{\textquoteright}ev, \{Aleksandr A.\} and Uvarov, \{Aleksandr V.\} and Komissarenko, \{Filipp E.\} and Mitin, \{Dmitry M.\} and Akanksha Kapoor and Joel Eymery and Nu{\~n}o Amador-Mendez and Christophe Durand and Dmitry Krasnikov and Nasibulin, \{Albert G.\} and Maria Tchernycheva and Mukhin, \{Ivan S.\}",

note = "Funding Information: The authors J.E., C.D. and A.K. would like to thank Jean Dussaud for his work on the MOVPE setup. V.N. would like to thank Maria Baeva for her assistance with the stretchable LED transparency measurements.J.E., C.D. and A.K. thank French National Labex GaNeX (ANR-11-LABX-0014) for MW synthesis and CL measurements. V.N. thanks the Russian Foundation for Basic Research (RFBR project no. 19-32-60040) for PDMS/MW membrane fabrication and optical measurements. I.S.M., V.N., F.M.K. thank the support from the Russian Science Foundation (grant 20-19-00256) for PDMS synthesis and electrical measurements. D.K. and A.G.N. thank Russian Foundation of Basic Research project no. 20-03-00804 for the synthesis of carbon nanotubes. F.E.K. thanks the support from the Russian Science Foundation (grant 19-79-00313) for the LED array encapsulation and membrane transfer. I.S.M., F.M.K., V.N., V.A.M., S.M., A.A.V., A.V.U., and D.A.M. thank the Ministry of Science and Higher Education of the Russian Federation (FSRM-2020-0005) for the general support. N.A. and M.T. acknowledge the financial support from the ITN Marie Curie project INDEED (grant no. 722176), by the Indo-French Centre for the Promotion of Advanced Research (IFCPAR/CEFIPRA project no. 6008-1) for MW/PDMS membrane processing and characterization. Funding Information: Funding: J.E., C.D. and A.K. thank French National Labex GaNeX (ANR-11-LABX-0014) for MW synthesis and CL measurements. V.N. thanks the Russian Foundation for Basic Research (RFBR project no. 19-32-60040) for PDMS/MW membrane fabrication and optical measurements. I.S.M., V.N., F.M.K. thank the support from the Russian Science Foundation (grant 20-19-00256) for PDMS synthesis and electrical measurements. D.K. and A.G.N. thank Russian Foundation of Basic Research project no. 20-03-00804 for the synthesis of carbon nanotubes. F.E.K. thanks the support from the Russian Science Foundation (grant 19-79-00313) for the LED array encapsulation and membrane transfer. I.S.M., F.M.K., V.N., V.A.M., S.M., A.A.V., A.V.U., and D.A.M. thank the Ministry of Science and Higher Education of the Russian Federation (FSRM-2020-0005) for the general support. N.A. and M.T. acknowledge the financial support from the ITN Marie Curie project INDEED (grant no. 722176), by the Indo-French Centre for the Promotion of Advanced Research (IFCPAR/CEFIPRA project no. 6008-1) for MW/PDMS membrane processing and characterization. Publisher Copyright: {\textcopyright} 2021 by the authors. Licensee MDPI, Basel, Switzerland.",

year = "2021",

month = jun,

doi = "10.3390/nano11061503",

language = "English",

volume = "11",

journal = "Nanomaterials",

issn = "2079-4991",

publisher = "MDPI AG",

number = "6",

}

Kochetkov, FM, Neplokh, V, Mastalieva, VA, Mukhangali, S, Vorob’ev, AA, Uvarov, AV, Komissarenko, FE, Mitin, DM, Kapoor, A, Eymery, J, Amador-Mendez, N, Durand, C, Krasnikov, D, Nasibulin, AG, Tchernycheva, M & Mukhin, IS 2021, 'Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films', Nanomaterials, Vuosikerta 11, Nro 6, 1503. https://doi.org/10.3390/nano11061503

TY - JOUR

T1 - Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films

AU - Kochetkov, Fedor M.

AU - Neplokh, Vladimir

AU - Mastalieva, Viktoria A.

AU - Mukhangali, Sungat

AU - Vorob’ev, Aleksandr A.

AU - Uvarov, Aleksandr V.

AU - Komissarenko, Filipp E.

AU - Mitin, Dmitry M.

AU - Kapoor, Akanksha

AU - Eymery, Joel

AU - Amador-Mendez, Nuño

AU - Durand, Christophe

AU - Krasnikov, Dmitry

AU - Nasibulin, Albert G.

AU - Tchernycheva, Maria

AU - Mukhin, Ivan S.

N1 - Funding Information: The authors J.E., C.D. and A.K. would like to thank Jean Dussaud for his work on the MOVPE setup. V.N. would like to thank Maria Baeva for her assistance with the stretchable LED transparency measurements.J.E., C.D. and A.K. thank French National Labex GaNeX (ANR-11-LABX-0014) for MW synthesis and CL measurements. V.N. thanks the Russian Foundation for Basic Research (RFBR project no. 19-32-60040) for PDMS/MW membrane fabrication and optical measurements. I.S.M., V.N., F.M.K. thank the support from the Russian Science Foundation (grant 20-19-00256) for PDMS synthesis and electrical measurements. D.K. and A.G.N. thank Russian Foundation of Basic Research project no. 20-03-00804 for the synthesis of carbon nanotubes. F.E.K. thanks the support from the Russian Science Foundation (grant 19-79-00313) for the LED array encapsulation and membrane transfer. I.S.M., F.M.K., V.N., V.A.M., S.M., A.A.V., A.V.U., and D.A.M. thank the Ministry of Science and Higher Education of the Russian Federation (FSRM-2020-0005) for the general support. N.A. and M.T. acknowledge the financial support from the ITN Marie Curie project INDEED (grant no. 722176), by the Indo-French Centre for the Promotion of Advanced Research (IFCPAR/CEFIPRA project no. 6008-1) for MW/PDMS membrane processing and characterization. Funding Information: Funding: J.E., C.D. and A.K. thank French National Labex GaNeX (ANR-11-LABX-0014) for MW synthesis and CL measurements. V.N. thanks the Russian Foundation for Basic Research (RFBR project no. 19-32-60040) for PDMS/MW membrane fabrication and optical measurements. I.S.M., V.N., F.M.K. thank the support from the Russian Science Foundation (grant 20-19-00256) for PDMS synthesis and electrical measurements. D.K. and A.G.N. thank Russian Foundation of Basic Research project no. 20-03-00804 for the synthesis of carbon nanotubes. F.E.K. thanks the support from the Russian Science Foundation (grant 19-79-00313) for the LED array encapsulation and membrane transfer. I.S.M., F.M.K., V.N., V.A.M., S.M., A.A.V., A.V.U., and D.A.M. thank the Ministry of Science and Higher Education of the Russian Federation (FSRM-2020-0005) for the general support. N.A. and M.T. acknowledge the financial support from the ITN Marie Curie project INDEED (grant no. 722176), by the Indo-French Centre for the Promotion of Advanced Research (IFCPAR/CEFIPRA project no. 6008-1) for MW/PDMS membrane processing and characterization. Publisher Copyright: © 2021 by the authors. Licensee MDPI, Basel, Switzerland.

PY - 2021/6

Y1 - 2021/6

N2 - We propose and demonstrate both flexible and stretchable blue light-emitting diodes based on core/shell InGaN/GaN quantum well microwires embedded in polydimethylsiloxane membranes with strain-insensitive transparent electrodes involving single-walled carbon nanotubes. InGaN/GaN core-shell microwires were grown by metal-organic vapor phase epitaxy, encapsulated into a polydimethylsiloxane film, and then released from the growth substrate. The fabricated free-standing membrane of light-emitting diodes with contacts of single-walled carbon nanotube films can stand up to 20% stretching while maintaining efficient operation. Membrane-based LEDs show less than 15% degradation of electroluminescence intensity after 20 cycles of stretching thus opening an avenue for highly deformable inorganic devices.

AB - We propose and demonstrate both flexible and stretchable blue light-emitting diodes based on core/shell InGaN/GaN quantum well microwires embedded in polydimethylsiloxane membranes with strain-insensitive transparent electrodes involving single-walled carbon nanotubes. InGaN/GaN core-shell microwires were grown by metal-organic vapor phase epitaxy, encapsulated into a polydimethylsiloxane film, and then released from the growth substrate. The fabricated free-standing membrane of light-emitting diodes with contacts of single-walled carbon nanotube films can stand up to 20% stretching while maintaining efficient operation. Membrane-based LEDs show less than 15% degradation of electroluminescence intensity after 20 cycles of stretching thus opening an avenue for highly deformable inorganic devices.

KW - InGaN

KW - MOVPE

KW - Nanowires

KW - Single-walled carbon nanotubes

KW - Stretchable LED

UR - https://www.scopus.com/pages/publications/85107285942

U2 - 10.3390/nano11061503

DO - 10.3390/nano11061503

M3 - Article

AN - SCOPUS:85107285942

SN - 2079-4991

VL - 11

JO - Nanomaterials

JF - Nanomaterials

IS - 6

M1 - 1503

ER -

Stretchable transparent light-emitting diodes based on ingan/gan quantum well microwires and carbon nanotube films

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