State-of-the-art luminescent materials based on wood veneer with superior strength, transparency, and water resistance

Ming Wang; Hongchen Liu; Xiao Feng; Xijun Wang; Kaiyuan Shen; Haisong Qi; Orlando J. Rojas

doi:10.1016/j.cej.2022.140225

State-of-the-art luminescent materials based on wood veneer with superior strength, transparency, and water resistance

Ming Wang, Hongchen Liu^*, Xiao Feng, Xijun Wang, Kaiyuan Shen, Haisong Qi^*, Orlando J. Rojas^*

^*Tämän työn vastaava kirjoittaja

Tutkimustuotos: Lehtiartikkeli › Article › Scientific › vertaisarvioitu

13 Sitaatiot (Scopus)

95 Lataukset (Pure)

Abstrakti

Current energy and luminescent materials utilize polymers to encapsulate fluorescent carbon nanodots and dyes but they usually lack stability and biodegradability. Here, we introduce an alternative wood nanotechnology to produce luminescent films (veneer) with UV resistance and tailorable surface energy. First, fluorescent and transparent wood (FTW) is shown as a support of aggregation-induced fluorescent emission (AIE) by in-situ Hantzsch reaction of acetoacetate delignified wood (AA-DW). Highly aligned cellulose nanofibers present in AA-DW facilitate FTW densification, ensuing exceptional mechanical performance (tensile strength and Young's modulus of up to 422 MPa and 45 GPa, respectively). Simultaneously, the conjugated structures display high transparency (83 %), haze (80 %) and optical anisotropy. The new luminescent system is demonstrated to be biodegradable and effective in optical (fluorescent) windows as well as encrypted films.

Alkuperäiskieli	Englanti
Artikkeli	140225
Julkaisu	Chemical Engineering Journal
Vuosikerta	454
Varhainen verkossa julkaisun päivämäärä	12 marrask. 2022
DOI - pysyväislinkit	https://doi.org/10.1016/j.cej.2022.140225
Tila	Julkaistu - 15 helmik. 2023
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

YK:n kestävän kehityksen tavoitteet

Tämä tuotos edistää seuraavia kestävän kehityksen tavoitteita:

Pääsy asiakirjaan

10.1016/j.cej.2022.140225Lisenssi: CC BY

CHEM_Wang_et_al_State-of-the-art_luminescent_2022_Chemical_Engineering_JournalFinal published version, 9,43 MBLisenssi: CC BY

Muut tiedostot ja linkit

Linkki julkaisuun Scopuksessa

BioELCell: Bioproducts Engineered from Lignocelluloses: from plants and upcycling to next generation materials
Rojas Gaona, O. (Vastuullinen tutkija), Abidnejad, R. (Projektin jäsen), Ajdary, R. (Projektin jäsen), Bhattarai, M. (Projektin jäsen), Zhu, Y. (Projektin jäsen), Zhao, B. (Projektin jäsen), Robertson, D. (Projektin jäsen), Reyes Torres, G. (Projektin jäsen), Johansson, L.-S. (Projektin jäsen), Garcia Greca, L. (Projektin jäsen), Klockars, K. (Projektin jäsen), Kämäräinen, T. (Projektin jäsen), Majoinen, J. (Projektin jäsen), Tardy, B. (Projektin jäsen), Dufau Mattos, B. (Projektin jäsen) & Ressouche, E. (Projektin jäsen)
30/07/2018 → 31/07/2023
Projekti: EU: ERC grants

Siteeraa tätä

@article{a11d5a6fdc744ad191e6114282875496,

title = "State-of-the-art luminescent materials based on wood veneer with superior strength, transparency, and water resistance",

abstract = "Current energy and luminescent materials utilize polymers to encapsulate fluorescent carbon nanodots and dyes but they usually lack stability and biodegradability. Here, we introduce an alternative wood nanotechnology to produce luminescent films (veneer) with UV resistance and tailorable surface energy. First, fluorescent and transparent wood (FTW) is shown as a support of aggregation-induced fluorescent emission (AIE) by in-situ Hantzsch reaction of acetoacetate delignified wood (AA-DW). Highly aligned cellulose nanofibers present in AA-DW facilitate FTW densification, ensuing exceptional mechanical performance (tensile strength and Young's modulus of up to 422 MPa and 45 GPa, respectively). Simultaneously, the conjugated structures display high transparency (83 %), haze (80 %) and optical anisotropy. The new luminescent system is demonstrated to be biodegradable and effective in optical (fluorescent) windows as well as encrypted films.",

keywords = "Aggregation-induced emission, Transparent wood, UV-blocking, Wood nanotechnology, Wood-based fluorescent films",

author = "Ming Wang and Hongchen Liu and Xiao Feng and Xijun Wang and Kaiyuan Shen and Haisong Qi and Rojas, {Orlando J.}",

note = "| openaire: EC/H2020/788489/EU//BioELCell Funding Information: The authors acknowledge funding support from the Guangdong Province Science Foundation (2017GC010429), the Guangdong Basic and Applied Basic Research Foundation (2022A1515010565), the Canada Excellence Research Chair Program (CERC-2018-00006), Canada Foundation for Innovation (Project number 38623) and the European Research Council (ERC) under the European Union{\textquoteright}s Horizon 2020 research and innovation programme (grant agreement No 788489, “BioElCell”). Dr. Xiaotong Fu (Jiangnan University) is thanked for WAXS data processing and Ayako Takagi (UBC) for designing the model house. ",

year = "2023",

month = feb,

day = "15",

doi = "10.1016/j.cej.2022.140225",

language = "English",

volume = "454",

journal = "Chemical Engineering Journal",

issn = "1385-8947",

publisher = "Elsevier Science Inc.",

}

TY - JOUR

T1 - State-of-the-art luminescent materials based on wood veneer with superior strength, transparency, and water resistance

AU - Wang, Ming

AU - Liu, Hongchen

AU - Feng, Xiao

AU - Wang, Xijun

AU - Shen, Kaiyuan

AU - Qi, Haisong

AU - Rojas, Orlando J.

N1 - | openaire: EC/H2020/788489/EU//BioELCell Funding Information: The authors acknowledge funding support from the Guangdong Province Science Foundation (2017GC010429), the Guangdong Basic and Applied Basic Research Foundation (2022A1515010565), the Canada Excellence Research Chair Program (CERC-2018-00006), Canada Foundation for Innovation (Project number 38623) and the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme (grant agreement No 788489, “BioElCell”). Dr. Xiaotong Fu (Jiangnan University) is thanked for WAXS data processing and Ayako Takagi (UBC) for designing the model house.

PY - 2023/2/15

Y1 - 2023/2/15

N2 - Current energy and luminescent materials utilize polymers to encapsulate fluorescent carbon nanodots and dyes but they usually lack stability and biodegradability. Here, we introduce an alternative wood nanotechnology to produce luminescent films (veneer) with UV resistance and tailorable surface energy. First, fluorescent and transparent wood (FTW) is shown as a support of aggregation-induced fluorescent emission (AIE) by in-situ Hantzsch reaction of acetoacetate delignified wood (AA-DW). Highly aligned cellulose nanofibers present in AA-DW facilitate FTW densification, ensuing exceptional mechanical performance (tensile strength and Young's modulus of up to 422 MPa and 45 GPa, respectively). Simultaneously, the conjugated structures display high transparency (83 %), haze (80 %) and optical anisotropy. The new luminescent system is demonstrated to be biodegradable and effective in optical (fluorescent) windows as well as encrypted films.

AB - Current energy and luminescent materials utilize polymers to encapsulate fluorescent carbon nanodots and dyes but they usually lack stability and biodegradability. Here, we introduce an alternative wood nanotechnology to produce luminescent films (veneer) with UV resistance and tailorable surface energy. First, fluorescent and transparent wood (FTW) is shown as a support of aggregation-induced fluorescent emission (AIE) by in-situ Hantzsch reaction of acetoacetate delignified wood (AA-DW). Highly aligned cellulose nanofibers present in AA-DW facilitate FTW densification, ensuing exceptional mechanical performance (tensile strength and Young's modulus of up to 422 MPa and 45 GPa, respectively). Simultaneously, the conjugated structures display high transparency (83 %), haze (80 %) and optical anisotropy. The new luminescent system is demonstrated to be biodegradable and effective in optical (fluorescent) windows as well as encrypted films.

KW - Aggregation-induced emission

KW - Transparent wood

KW - UV-blocking

KW - Wood nanotechnology

KW - Wood-based fluorescent films

UR - http://www.scopus.com/inward/record.url?scp=85141751344&partnerID=8YFLogxK

U2 - 10.1016/j.cej.2022.140225

DO - 10.1016/j.cej.2022.140225

M3 - Article

AN - SCOPUS:85141751344

SN - 1385-8947

VL - 454

JO - Chemical Engineering Journal

JF - Chemical Engineering Journal

M1 - 140225

ER -

State-of-the-art luminescent materials based on wood veneer with superior strength, transparency, and water resistance

Abstrakti

YK:n kestävän kehityksen tavoitteet

Pääsy asiakirjaan

Muut tiedostot ja linkit

Sormenjälki

Projektit

BioELCell: Bioproducts Engineered from Lignocelluloses: from plants and upcycling to next generation materials

Siteeraa tätä