Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films

Alan Farhan; Maria Cocconcelli; Federico Stramaglia; Nikolai Kuznetsov; Lukáš Flajšman; Marcus Wyss; Lide Yao; Cinthia Piamonteze; Sebastiaan Van Dijken

doi:10.1103/PhysRevMaterials.7.044402

Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films

Alan Farhan, Maria Cocconcelli, Federico Stramaglia, Nikolai Kuznetsov, Lukáš Flajšman, Marcus Wyss, Lide Yao, Cinthia Piamonteze, Sebastiaan Van Dijken

Tutkimustuotos: Lehtiartikkeli › Article › Scientific › vertaisarvioitu

7 Sitaatiot (Scopus)

76 Lataukset (Pure)

Abstrakti

We present a study on the structural and magnetic properties of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 (Lu5BO) high-entropy oxide perovskite thin films. We use synchrotron-based x-ray absorption spectroscopy employing x-ray magnetic circular and linear dichroism (XMCD and XMLD) to perform an element-sensitive study on single-crystal epitaxial Lu5BO thin films. Together with XMCD magnetometry, the results reveal dominant antiferromagnetic order with a transition temperature around 100 K.

Alkuperäiskieli	Englanti
Artikkeli	044402
Sivut	1-7
Sivumäärä	7
Julkaisu	Physical Review Materials
Vuosikerta	7
Numero	4
DOI - pysyväislinkit	https://doi.org/10.1103/PhysRevMaterials.7.044402
Tila	Julkaistu - huhtik. 2023
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Pääsy asiakirjaan

10.1103/PhysRevMaterials.7.044402

Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 high-entropy oxide perovskite thin filmsFinal published version, 1,82 MB

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Sähköisten, magneettisten ja plasmonisten nanomateriaalien ioninen ohjaus
van Dijken, S. (Vastuullinen tutkija), Freire Fernandez, F. (Projektin jäsen), Perumbilavil, S. (Projektin jäsen), Lepikko, S. (Projektin jäsen), Farhan, A. (Projektin jäsen), Hagnäs, R. (Projektin jäsen) & Ameziane, M. (Projektin jäsen)
01/09/2018 → 31/08/2022
Projekti: Academy of Finland: Other research funding

OtaNano
Rissanen, A. (Manager)
Aalto-yliopisto
Laitteistot/tilat: Facility
OtaNano Nanomikroskopiakeskus
Seitsonen, J. (Manager) & Rissanen, A. (Other)
OtaNano
Laitteistot/tilat: Facility

Siteeraa tätä

Farhan, A., Cocconcelli, M., Stramaglia, F., Kuznetsov, N., Flajšman, L., Wyss, M., Yao, L., Piamonteze, C., & Van Dijken, S. (2023). Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films. Physical Review Materials, 7(4), 1-7. Artikkeli 044402. https://doi.org/10.1103/PhysRevMaterials.7.044402

@article{19a742d467474620a13aa6886a222f44,

title = "Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films",

abstract = "We present a study on the structural and magnetic properties of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 (Lu5BO) high-entropy oxide perovskite thin films. We use synchrotron-based x-ray absorption spectroscopy employing x-ray magnetic circular and linear dichroism (XMCD and XMLD) to perform an element-sensitive study on single-crystal epitaxial Lu5BO thin films. Together with XMCD magnetometry, the results reveal dominant antiferromagnetic order with a transition temperature around 100 K.",

author = "Alan Farhan and Maria Cocconcelli and Federico Stramaglia and Nikolai Kuznetsov and Luk{\'a}{\v s} Flaj{\v s}man and Marcus Wyss and Lide Yao and Cinthia Piamonteze and {Van Dijken}, Sebastiaan",

note = "Funding Information: The authors thank A. Kleibert and Y.-L. Huang for their support and fruitful discussions. This work was supported by the Academy of Finland (Project No. 316857) and part of this work was performed at the XTreme beamline of the Swiss Light Source. F.S. is funded by the Swiss National Science Foundation (SNF) (Grant No. 200021_184684). SQUID-VSM measurements were carried out on the Quantum Design MPMS3-137 device of the Laboratory for Mesoscopic Systems, ETH Zurich, Switzerland and the Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Switzerland. We acknowledge the provision of facilities and technical support by Aalto University at OtaNano - Nanomicroscopy Center (Aalto-NMC). Publisher Copyright: {\textcopyright} 2023 American Physical Society.",

year = "2023",

month = apr,

doi = "10.1103/PhysRevMaterials.7.044402",

language = "English",

volume = "7",

pages = "1--7",

journal = "Physical Review Materials",

issn = "2475-9953",

publisher = "American Physical Society",

number = "4",

}

Farhan, A, Cocconcelli, M, Stramaglia, F, Kuznetsov, N, Flajšman, L, Wyss, M, Yao, L, Piamonteze, C & Van Dijken, S 2023, 'Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films', Physical Review Materials, Vuosikerta 7, Nro 4, 044402, Sivut 1-7. https://doi.org/10.1103/PhysRevMaterials.7.044402

TY - JOUR

T1 - Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films

AU - Farhan, Alan

AU - Cocconcelli, Maria

AU - Stramaglia, Federico

AU - Kuznetsov, Nikolai

AU - Flajšman, Lukáš

AU - Wyss, Marcus

AU - Yao, Lide

AU - Piamonteze, Cinthia

AU - Van Dijken, Sebastiaan

N1 - Funding Information: The authors thank A. Kleibert and Y.-L. Huang for their support and fruitful discussions. This work was supported by the Academy of Finland (Project No. 316857) and part of this work was performed at the XTreme beamline of the Swiss Light Source. F.S. is funded by the Swiss National Science Foundation (SNF) (Grant No. 200021_184684). SQUID-VSM measurements were carried out on the Quantum Design MPMS3-137 device of the Laboratory for Mesoscopic Systems, ETH Zurich, Switzerland and the Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Switzerland. We acknowledge the provision of facilities and technical support by Aalto University at OtaNano - Nanomicroscopy Center (Aalto-NMC). Publisher Copyright: © 2023 American Physical Society.

PY - 2023/4

Y1 - 2023/4

N2 - We present a study on the structural and magnetic properties of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 (Lu5BO) high-entropy oxide perovskite thin films. We use synchrotron-based x-ray absorption spectroscopy employing x-ray magnetic circular and linear dichroism (XMCD and XMLD) to perform an element-sensitive study on single-crystal epitaxial Lu5BO thin films. Together with XMCD magnetometry, the results reveal dominant antiferromagnetic order with a transition temperature around 100 K.

AB - We present a study on the structural and magnetic properties of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 (Lu5BO) high-entropy oxide perovskite thin films. We use synchrotron-based x-ray absorption spectroscopy employing x-ray magnetic circular and linear dichroism (XMCD and XMLD) to perform an element-sensitive study on single-crystal epitaxial Lu5BO thin films. Together with XMCD magnetometry, the results reveal dominant antiferromagnetic order with a transition temperature around 100 K.

UR - http://www.scopus.com/inward/record.url?scp=85153478253&partnerID=8YFLogxK

U2 - 10.1103/PhysRevMaterials.7.044402

DO - 10.1103/PhysRevMaterials.7.044402

M3 - Article

AN - SCOPUS:85153478253

SN - 2475-9953

VL - 7

SP - 1

EP - 7

JO - Physical Review Materials

JF - Physical Review Materials

IS - 4

M1 - 044402

ER -

Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films

Abstrakti

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Muut tiedostot ja linkit

Sormenjälki

Projektit

Sähköisten, magneettisten ja plasmonisten nanomateriaalien ioninen ohjaus

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OtaNano

OtaNano Nanomikroskopiakeskus

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