Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook

Jiaqi Wang; Yongdan Li; Christin Hummel; Guo Huang; Xiaoyan Ji; Ezgi Demiröz; Atsushi Urakawa; Siyuan Huang; Ruixue Zhao; Johannes Lercher; Paola Lanzafame; Georgia Papanikolaou; Gabriele Centi

doi:10.1021/acs.energyfuels.4c04644

Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook

Jiaqi Wang, Yongdan Li, Christin Hummel, Guo Huang, Xiaoyan Ji^*, Ezgi Demiröz, Atsushi Urakawa, Siyuan Huang, Ruixue Zhao, Johannes Lercher, Paola Lanzafame, Georgia Papanikolaou, Gabriele Centi^*

^*Tämän työn vastaava kirjoittaja

Tutkimustuotos: Lehtiartikkeli › Review Article › vertaisarvioitu

13 Lataukset (Pure)

Abstrakti

Green hydrogen plays a crucial role in decarbonization and the future of low-carbon society. Still, its transport/distribution and cost of production, mainly realized by electrolysis, are major hurdles. Liquid H₂ carriers reduce transport/distribution costs but add further expenses for their production. To address this challenge, we proposed a novel strategy for electrocatalytic production of a liquid organic hydrogen carrier with anodic valorization of the process. This review summarizes the state of the art and outlooks in this new concept. The electrocatalytic process is briefly introduced, and the main components are discussed. Subsequently, the electrocatalytic production of liquid organic hydrogen carriers and anodic oxidation from components to processes, together with the paired processes and reactors, are analyzed, highlighting challenges and prospects.

Alkuperäiskieli	Englanti
Sivut	132–165
Julkaisu	Energy and Fuels
Vuosikerta	39
Numero	1
Varhainen verkossa julkaisun päivämäärä	25 jouluk. 2024
DOI - pysyväislinkit	https://doi.org/10.1021/acs.energyfuels.4c04644
Tila	Julkaistu - 9 tammik. 2025
OKM-julkaisutyyppi	A2 Katsausartikkeli tieteellisessä aikakauslehdessä

YK:n kestävän kehityksen tavoitteet

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10.1021/acs.energyfuels.4c04644Lisenssi: CC BY

CHEM_Wang_et_al_Electrocatalytic_Production_2025_Energy_FuelsFinal published version, 5,23 MBLisenssi: CC BY

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Linkki julkaisuun Scopuksessa

EPOCH, Teke: Electrocatalytic Production of liquid Organic hydrogen carrier and CHemicals from lignin
Li, Y. (Vastuullinen tutkija)
01/10/2022 → 30/09/2026
Projekti: EU: Framework programmes funding

Siteeraa tätä

Wang, J., Li, Y., Hummel, C., Huang, G., Ji, X., Demiröz, E., Urakawa, A., Huang, S., Zhao, R., Lercher, J., Lanzafame, P., Papanikolaou, G., & Centi, G. (2025). Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook. Energy and Fuels, 39(1), 132–165. https://doi.org/10.1021/acs.energyfuels.4c04644

@article{07a34b8c8ccd4189a8ad11597ae3d3e3,

title = "Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook",

abstract = "Green hydrogen plays a crucial role in decarbonization and the future of low-carbon society. Still, its transport/distribution and cost of production, mainly realized by electrolysis, are major hurdles. Liquid H2 carriers reduce transport/distribution costs but add further expenses for their production. To address this challenge, we proposed a novel strategy for electrocatalytic production of a liquid organic hydrogen carrier with anodic valorization of the process. This review summarizes the state of the art and outlooks in this new concept. The electrocatalytic process is briefly introduced, and the main components are discussed. Subsequently, the electrocatalytic production of liquid organic hydrogen carriers and anodic oxidation from components to processes, together with the paired processes and reactors, are analyzed, highlighting challenges and prospects.",

author = "Jiaqi Wang and Yongdan Li and Christin Hummel and Guo Huang and Xiaoyan Ji and Ezgi Demir{\"o}z and Atsushi Urakawa and Siyuan Huang and Ruixue Zhao and Johannes Lercher and Paola Lanzafame and Georgia Papanikolaou and Gabriele Centi",

note = "| openaire: EC/HE/101070976/EU//EPOCH",

year = "2025",

month = jan,

day = "9",

doi = "10.1021/acs.energyfuels.4c04644",

language = "English",

volume = "39",

pages = "132–165",

journal = "Energy and Fuels",

issn = "0887-0624",

publisher = "American Chemical Society",

number = "1",

}

Wang, J, Li, Y, Hummel, C, Huang, G, Ji, X, Demiröz, E, Urakawa, A, Huang, S, Zhao, R, Lercher, J, Lanzafame, P, Papanikolaou, G & Centi, G 2025, 'Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook', Energy and Fuels, Vuosikerta 39, Nro 1, Sivut 132–165. https://doi.org/10.1021/acs.energyfuels.4c04644

TY - JOUR

T1 - Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook

AU - Wang, Jiaqi

AU - Li, Yongdan

AU - Hummel, Christin

AU - Huang, Guo

AU - Ji, Xiaoyan

AU - Demiröz, Ezgi

AU - Urakawa, Atsushi

AU - Huang, Siyuan

AU - Zhao, Ruixue

AU - Lercher, Johannes

AU - Lanzafame, Paola

AU - Papanikolaou, Georgia

AU - Centi, Gabriele

N1 - | openaire: EC/HE/101070976/EU//EPOCH

PY - 2025/1/9

Y1 - 2025/1/9

N2 - Green hydrogen plays a crucial role in decarbonization and the future of low-carbon society. Still, its transport/distribution and cost of production, mainly realized by electrolysis, are major hurdles. Liquid H2 carriers reduce transport/distribution costs but add further expenses for their production. To address this challenge, we proposed a novel strategy for electrocatalytic production of a liquid organic hydrogen carrier with anodic valorization of the process. This review summarizes the state of the art and outlooks in this new concept. The electrocatalytic process is briefly introduced, and the main components are discussed. Subsequently, the electrocatalytic production of liquid organic hydrogen carriers and anodic oxidation from components to processes, together with the paired processes and reactors, are analyzed, highlighting challenges and prospects.

AB - Green hydrogen plays a crucial role in decarbonization and the future of low-carbon society. Still, its transport/distribution and cost of production, mainly realized by electrolysis, are major hurdles. Liquid H2 carriers reduce transport/distribution costs but add further expenses for their production. To address this challenge, we proposed a novel strategy for electrocatalytic production of a liquid organic hydrogen carrier with anodic valorization of the process. This review summarizes the state of the art and outlooks in this new concept. The electrocatalytic process is briefly introduced, and the main components are discussed. Subsequently, the electrocatalytic production of liquid organic hydrogen carriers and anodic oxidation from components to processes, together with the paired processes and reactors, are analyzed, highlighting challenges and prospects.

UR - http://www.scopus.com/inward/record.url?scp=85213230318&partnerID=8YFLogxK

U2 - 10.1021/acs.energyfuels.4c04644

DO - 10.1021/acs.energyfuels.4c04644

M3 - Review Article

AN - SCOPUS:85213230318

SN - 0887-0624

VL - 39

SP - 132

EP - 165

JO - Energy and Fuels

JF - Energy and Fuels

IS - 1

ER -

Electrocatalytic Production of a Liquid Organic Hydrogen Carrier with Anodic Valorization of the Process: Review and Outlook

Abstrakti

YK:n kestävän kehityksen tavoitteet

Pääsy asiakirjaan

Muut tiedostot ja linkit

Sormenjälki

Projektit

EPOCH, Teke: Electrocatalytic Production of liquid Organic hydrogen carrier and CHemicals from lignin

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