Additive Manufacturing of Single-Layer Protonic Ceramic Fuel Cells

Imran Asghar; Peter Lund

doi:10.1149/11106.1927ecst

Additive Manufacturing of Single-Layer Protonic Ceramic Fuel Cells

Tutkimustuotos: Lehtiartikkeli › Conference article › Scientific › vertaisarvioitu

Abstrakti

Single-layer proton conducting ceramic fuel cells (PCFCs) were fabricated through a hybrid of extrusion-based 3D printing utilizing BaZr0.4Ce0.4Y0.1Yb0.1O3-δ (BZCYYb) as an ionic conductor, and BaCo0.4Fe0.4Zr0.1Y0.1O3-δ (BCFZY) as the electrode material. The rheological properties of the printable pastes were investigated in detail. The 3D printed single-layer cell produced a maximum power density of 283 mW/cm2 at 550oC. The performance was mainly limited due to limited surface area on both sides of the cell. The performance improved by 17% (331 mW/cm2) when porous layers were added on both sides of the cell. In addition, cells with traditional 3-layer structure were fabricated using NiO-BZCYYb as anode, BZCYYb as electrolyte, and BCFZY-BZCYYb as cathode. The cell produced a maximum power density of 426 mW/cm2 at 650OC. The performance improved by 120% (938 mW/cm2) when a composite of BZCYYb and a eutectic mixture of Li2CO3, Na2CO3 and K2CO3 was used as electrolyte.

Alkuperäiskieli	Englanti
Sivut	1927-1931
Julkaisu	ECS Transactions
Vuosikerta	111
Numero	6
DOI - pysyväislinkit	https://doi.org/10.1149/11106.1927ecst
Tila	Julkaistu - 2023
OKM-julkaisutyyppi	A4 Artikkeli konferenssijulkaisussa
Tapahtuma	International Symposium on Solid Oxide Fuel Cells - Boston, Yhdysvallat Kesto: 28 toukok. 2023 → 2 kesäk. 2023 Konferenssinumero: 18

Pääsy asiakirjaan

10.1149/11106.1927ecst

Leading-edge next generation fuel cell devices
Asghar, I. (Vastuullinen johtaja), Zarabi Golkhatmi, S. (Projektin jäsen) & Virtanen, S. (Projektin jäsen)
01/09/2022 → 31/08/2024
Projekti: RCF Academy Research Fellow: Research costs
Seuraavan sukupolven johtavat polttokennot
Asghar, I. (Vastuullinen johtaja), Bilbey, B. (Projektin jäsen), Zarabi Golkhatmi, S. (Projektin jäsen), Jouttijärvi, S. (Projektin jäsen), Virtanen, S. (Projektin jäsen), Jokinen, A. (Projektin jäsen), Markkanen, M. (Projektin jäsen), Savikko, A. (Projektin jäsen) & Mäkinen, P. (Projektin jäsen)
01/09/2019 → 31/08/2022
Projekti: Academy of Finland: Other research funding

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@article{3076b2d7138b4b6e932647124f9ac57e,

title = "Additive Manufacturing of Single-Layer Protonic Ceramic Fuel Cells",

abstract = "Single-layer proton conducting ceramic fuel cells (PCFCs) were fabricated through a hybrid of extrusion-based 3D printing utilizing BaZr0.4Ce0.4Y0.1Yb0.1O3-δ (BZCYYb) as an ionic conductor, and BaCo0.4Fe0.4Zr0.1Y0.1O3-δ (BCFZY) as the electrode material. The rheological properties of the printable pastes were investigated in detail. The 3D printed single-layer cell produced a maximum power density of 283 mW/cm2 at 550oC. The performance was mainly limited due to limited surface area on both sides of the cell. The performance improved by 17\% (331 mW/cm2) when porous layers were added on both sides of the cell. In addition, cells with traditional 3-layer structure were fabricated using NiO-BZCYYb as anode, BZCYYb as electrolyte, and BCFZY-BZCYYb as cathode. The cell produced a maximum power density of 426 mW/cm2 at 650OC. The performance improved by 120\% (938 mW/cm2) when a composite of BZCYYb and a eutectic mixture of Li2CO3, Na2CO3 and K2CO3 was used as electrolyte.",

author = "Imran Asghar and Peter Lund",

year = "2023",

doi = "10.1149/11106.1927ecst",

language = "English",

volume = "111",

pages = "1927--1931",

journal = "ECS Transactions",

issn = "1938-5862",

publisher = "Institute of Physics Publishing",

number = "6",

note = "International Symposium on Solid Oxide Fuel Cells, SOFC ; Conference date: 28-05-2023 Through 02-06-2023",

}

TY - JOUR

T1 - Additive Manufacturing of Single-Layer Protonic Ceramic Fuel Cells

AU - Asghar, Imran

AU - Lund, Peter

N1 - Conference code: 18

PY - 2023

Y1 - 2023

N2 - Single-layer proton conducting ceramic fuel cells (PCFCs) were fabricated through a hybrid of extrusion-based 3D printing utilizing BaZr0.4Ce0.4Y0.1Yb0.1O3-δ (BZCYYb) as an ionic conductor, and BaCo0.4Fe0.4Zr0.1Y0.1O3-δ (BCFZY) as the electrode material. The rheological properties of the printable pastes were investigated in detail. The 3D printed single-layer cell produced a maximum power density of 283 mW/cm2 at 550oC. The performance was mainly limited due to limited surface area on both sides of the cell. The performance improved by 17% (331 mW/cm2) when porous layers were added on both sides of the cell. In addition, cells with traditional 3-layer structure were fabricated using NiO-BZCYYb as anode, BZCYYb as electrolyte, and BCFZY-BZCYYb as cathode. The cell produced a maximum power density of 426 mW/cm2 at 650OC. The performance improved by 120% (938 mW/cm2) when a composite of BZCYYb and a eutectic mixture of Li2CO3, Na2CO3 and K2CO3 was used as electrolyte.

AB - Single-layer proton conducting ceramic fuel cells (PCFCs) were fabricated through a hybrid of extrusion-based 3D printing utilizing BaZr0.4Ce0.4Y0.1Yb0.1O3-δ (BZCYYb) as an ionic conductor, and BaCo0.4Fe0.4Zr0.1Y0.1O3-δ (BCFZY) as the electrode material. The rheological properties of the printable pastes were investigated in detail. The 3D printed single-layer cell produced a maximum power density of 283 mW/cm2 at 550oC. The performance was mainly limited due to limited surface area on both sides of the cell. The performance improved by 17% (331 mW/cm2) when porous layers were added on both sides of the cell. In addition, cells with traditional 3-layer structure were fabricated using NiO-BZCYYb as anode, BZCYYb as electrolyte, and BCFZY-BZCYYb as cathode. The cell produced a maximum power density of 426 mW/cm2 at 650OC. The performance improved by 120% (938 mW/cm2) when a composite of BZCYYb and a eutectic mixture of Li2CO3, Na2CO3 and K2CO3 was used as electrolyte.

U2 - 10.1149/11106.1927ecst

DO - 10.1149/11106.1927ecst

M3 - Conference article

SN - 1938-5862

VL - 111

SP - 1927

EP - 1931

JO - ECS Transactions

JF - ECS Transactions

IS - 6

T2 - International Symposium on Solid Oxide Fuel Cells

Y2 - 28 May 2023 through 2 June 2023

ER -

Additive Manufacturing of Single-Layer Protonic Ceramic Fuel Cells

Abstrakti

Pääsy asiakirjaan

Sormenjälki

Projektit

Leading-edge next generation fuel cell devices

Seuraavan sukupolven johtavat polttokennot

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