A general ink formulation of 2D crystals for wafer-scale inkjet printing

Guohua Hu; Lisong Yang; Zongyin Yang; Yubo Wang; Xinxin Jin; Jie Dai; Qing Wu; Shouhu Liu; Xiaoxi Zhu; Xiaoshan Wang; Tien Chun Wu; Richard C.T. Howe; Tom Albrow-Owen; Leonard W.T. Ng; Qing Yang; Luigi G. Occhipinti; Robert I. Woodward; Edmund J.R. Kelleher; Zhipei Sun; Xiao Huang; Meng Zhang; Colin D. Bain; Tawfique Hasan

doi:10.1126/sciadv.aba5029

A general ink formulation of 2D crystals for wafer-scale inkjet printing

Guohua Hu, Lisong Yang, Zongyin Yang, Yubo Wang, Xinxin Jin, Jie Dai, Qing Wu, Shouhu Liu, Xiaoxi Zhu, Xiaoshan Wang, Tien Chun Wu, Richard C.T. Howe, Tom Albrow-Owen, Leonard W.T. Ng, Qing Yang, Luigi G. Occhipinti, Robert I. Woodward, Edmund J.R. Kelleher, Zhipei Sun, Xiao HuangMeng Zhang, Colin D. Bain, Tawfique Hasan

Tutkimustuotos: Lehtiartikkeli › Article › Scientific › vertaisarvioitu

112 Sitaatiot (Scopus)

90 Lataukset (Pure)

Abstrakti

Recent advances in inkjet printing of two-dimensional (2D) crystals show great promise for next-generation printed electronics development. Printing nonuniformity, however, results in poor reproducibility in device performance and remains a major impediment to their large-scale manufacturing. At the heart of this challenge lies the coffee-ring effect (CRE), ring-shaped nonuniform deposits formed during postdeposition drying. We present an experimental study of the drying mechanism of a binary solvent ink formulation. We show that Marangoni-enhanced spreading in this formulation inhibits contact line pinning and deforms the droplet shape to naturally suppress the capillary flows that give rise to the CRE. This general formulation supports uniform deposition of 2D crystals and their derivatives, enabling scalable and even wafer-scale device fabrication, moving them closer to industrial-level additive manufacturing.

Alkuperäiskieli	Englanti
Artikkeli	eaba5029
Sivut	eaba5029
Sivumäärä	6
Julkaisu	Science Advances
Vuosikerta	6
Numero	33
DOI - pysyväislinkit	https://doi.org/10.1126/sciadv.aba5029
Tila	Julkaistu - 1 elok. 2020
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Pääsy asiakirjaan

10.1126/sciadv.aba5029Lisenssi: CC BY

Hu_General_ink_formulation_of_2d_crystals_ScAdFinal published version, 9,38 MBLisenssi: CC BY

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Link to publication in Scopus

1 Aktiivinen
2 Päättynyt

-: Atomically-engineered nonlinear photonics with two-dimensional layered superlattices.
Sun, Z. (Vastuullinen tutkija), Varjamo, S.-T. (Projektin jäsen), Wang, Y. (Projektin jäsen), Pelgrin, V. (Projektin jäsen), Wang, Y. (Projektin jäsen), Yoon, H. H. (Projektin jäsen), Das, S. (Projektin jäsen), Huang, Y. (Projektin jäsen), Liapis, A. (Projektin jäsen), Dai, Y. (Projektin jäsen), Mohsen, A. (Projektin jäsen), Nigmatulin, F. (Projektin jäsen), Uddin, M. (Projektin jäsen), Du, M. (Projektin jäsen), Zhang, Y. (Projektin jäsen), Arias, J. C. (Projektin jäsen), Lin, Y. (Projektin jäsen), Pajunpää, T. (Projektin jäsen), Turunen, M. (Projektin jäsen), Cui, X. (Projektin jäsen), Xing, J. (Projektin jäsen), Cheng, X. (Projektin jäsen), Kaaripuro, H. (Projektin jäsen), Edwards, C. (Projektin jäsen) & Shahin, R. A. (Projektin jäsen)
01/09/2019 → 31/08/2025
Projekti: EU: ERC grants
A-Photonics
Sun, Z. (Vastuullinen tutkija), Pyymaki Perros, A. (Projektin jäsen), Kuen Yao, L. (Projektin jäsen), Rajamanickam, R. (Projektin jäsen), Dai, Y. (Projektin jäsen), Du, M. (Projektin jäsen), Kim, M. (Projektin jäsen) & Hedberg, D. (Projektin jäsen)
01/01/2019 → 31/12/2020
Projekti: Business Finland: New business from research ideas (TUTLI)
S2QUIP: Scalable Two-Dimensional Quantum Integrated Photonics
Sun, Z. (Vastuullinen tutkija), Wang, Y. (Projektin jäsen), Du, M. (Projektin jäsen), Uddin, M. (Projektin jäsen), Mohsen, A. (Projektin jäsen), Hu, X. (Projektin jäsen), Bai, X. (Projektin jäsen), Yoon, H. H. (Projektin jäsen) & Turunen, M. (Projektin jäsen)
01/10/2018 → 31/03/2022
Projekti: EU: Framework programmes funding

Siteeraa tätä

Hu, G., Yang, L., Yang, Z., Wang, Y., Jin, X., Dai, J., Wu, Q., Liu, S., Zhu, X., Wang, X., Wu, T. C., Howe, R. C. T., Albrow-Owen, T., Ng, L. W. T., Yang, Q., Occhipinti, L. G., Woodward, R. I., Kelleher, E. J. R., Sun, Z., ... Hasan, T. (2020). A general ink formulation of 2D crystals for wafer-scale inkjet printing. Science Advances, 6(33), eaba5029. Artikkeli eaba5029. https://doi.org/10.1126/sciadv.aba5029

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title = "A general ink formulation of 2D crystals for wafer-scale inkjet printing",

abstract = "Recent advances in inkjet printing of two-dimensional (2D) crystals show great promise for next-generation printed electronics development. Printing nonuniformity, however, results in poor reproducibility in device performance and remains a major impediment to their large-scale manufacturing. At the heart of this challenge lies the coffee-ring effect (CRE), ring-shaped nonuniform deposits formed during postdeposition drying. We present an experimental study of the drying mechanism of a binary solvent ink formulation. We show that Marangoni-enhanced spreading in this formulation inhibits contact line pinning and deforms the droplet shape to naturally suppress the capillary flows that give rise to the CRE. This general formulation supports uniform deposition of 2D crystals and their derivatives, enabling scalable and even wafer-scale device fabrication, moving them closer to industrial-level additive manufacturing.",

author = "Guohua Hu and Lisong Yang and Zongyin Yang and Yubo Wang and Xinxin Jin and Jie Dai and Qing Wu and Shouhu Liu and Xiaoxi Zhu and Xiaoshan Wang and Wu, {Tien Chun} and Howe, {Richard C.T.} and Tom Albrow-Owen and Ng, {Leonard W.T.} and Qing Yang and Occhipinti, {Luigi G.} and Woodward, {Robert I.} and Kelleher, {Edmund J.R.} and Zhipei Sun and Xiao Huang and Meng Zhang and Bain, {Colin D.} and Tawfique Hasan",

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Hu, G, Yang, L, Yang, Z, Wang, Y, Jin, X, Dai, J, Wu, Q, Liu, S, Zhu, X, Wang, X, Wu, TC, Howe, RCT, Albrow-Owen, T, Ng, LWT, Yang, Q, Occhipinti, LG, Woodward, RI, Kelleher, EJR, Sun, Z, Huang, X, Zhang, M, Bain, CD & Hasan, T 2020, 'A general ink formulation of 2D crystals for wafer-scale inkjet printing', Science Advances, Vuosikerta 6, Nro 33, eaba5029, Sivut eaba5029. https://doi.org/10.1126/sciadv.aba5029

TY - JOUR

T1 - A general ink formulation of 2D crystals for wafer-scale inkjet printing

AU - Hu, Guohua

AU - Yang, Lisong

AU - Yang, Zongyin

AU - Wang, Yubo

AU - Jin, Xinxin

AU - Dai, Jie

AU - Wu, Qing

AU - Liu, Shouhu

AU - Zhu, Xiaoxi

AU - Wang, Xiaoshan

AU - Wu, Tien Chun

AU - Howe, Richard C.T.

AU - Albrow-Owen, Tom

AU - Ng, Leonard W.T.

AU - Yang, Qing

AU - Occhipinti, Luigi G.

AU - Woodward, Robert I.

AU - Kelleher, Edmund J.R.

AU - Sun, Zhipei

AU - Huang, Xiao

AU - Zhang, Meng

AU - Bain, Colin D.

AU - Hasan, Tawfique

N1 - | openaire: EC/H2020/834742/EU//ATOP | openaire: EC/H2020/820423/EU//S2QUIP

PY - 2020/8/1

Y1 - 2020/8/1

N2 - Recent advances in inkjet printing of two-dimensional (2D) crystals show great promise for next-generation printed electronics development. Printing nonuniformity, however, results in poor reproducibility in device performance and remains a major impediment to their large-scale manufacturing. At the heart of this challenge lies the coffee-ring effect (CRE), ring-shaped nonuniform deposits formed during postdeposition drying. We present an experimental study of the drying mechanism of a binary solvent ink formulation. We show that Marangoni-enhanced spreading in this formulation inhibits contact line pinning and deforms the droplet shape to naturally suppress the capillary flows that give rise to the CRE. This general formulation supports uniform deposition of 2D crystals and their derivatives, enabling scalable and even wafer-scale device fabrication, moving them closer to industrial-level additive manufacturing.

AB - Recent advances in inkjet printing of two-dimensional (2D) crystals show great promise for next-generation printed electronics development. Printing nonuniformity, however, results in poor reproducibility in device performance and remains a major impediment to their large-scale manufacturing. At the heart of this challenge lies the coffee-ring effect (CRE), ring-shaped nonuniform deposits formed during postdeposition drying. We present an experimental study of the drying mechanism of a binary solvent ink formulation. We show that Marangoni-enhanced spreading in this formulation inhibits contact line pinning and deforms the droplet shape to naturally suppress the capillary flows that give rise to the CRE. This general formulation supports uniform deposition of 2D crystals and their derivatives, enabling scalable and even wafer-scale device fabrication, moving them closer to industrial-level additive manufacturing.

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SN - 2375-2548

VL - 6

SP - eaba5029

JO - Science Advances

JF - Science Advances

IS - 33

M1 - eaba5029

ER -

A general ink formulation of 2D crystals for wafer-scale inkjet printing

Abstrakti

Pääsy asiakirjaan

Muut tiedostot ja linkit

Sormenjälki

Projektit

-: Atomically-engineered nonlinear photonics with two-dimensional layered superlattices.

A-Photonics

S2QUIP: Scalable Two-Dimensional Quantum Integrated Photonics

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