Understanding Nanocellulose-Water Interactions: Turning a Detriment into an Asset

Laleh Solhi; Valentina Guccini; Katja Heise; Iina Solala; Elina Niinivaara; Wenyang Xu; Karl Mihhels; Marcel Kröger; Zhuojun Meng; Jakob Wohlert; Han Tao; Emily D. Cranston; Eero Kontturi

doi:10.1021/acs.chemrev.2c00611

Understanding Nanocellulose-Water Interactions: Turning a Detriment into an Asset

Laleh Solhi^*
, Valentina Guccini^*
, Katja Heise
, Iina Solala
, Elina Niinivaara
, Wenyang Xu
, Karl Mihhels
, Marcel Kröger
, Zhuojun Meng
, Jakob Wohlert
, Han Tao
, Emily D. Cranston
, Eero Kontturi^*

^*Corresponding author for this work

University of British Columbia
Åbo Akademi University
University of Chinese Academy of Sciences
KTH Royal Institute of Technology

Research output: Contribution to journal › Review Article › peer-review

456 Citations (Scopus)

677 Downloads (Pure)

Abstract

Modern technology has enabled the isolation of nanocellulose from plant-based fibers, and the current trend focuses on utilizing nanocellulose in a broad range of sustainable materials applications. Water is generally seen as a detrimental component when in contact with nanocellulose-based materials, just like it is harmful for traditional cellulosic materials such as paper or cardboard. However, water is an integral component in plants, and many applications of nanocellulose already accept the presence of water or make use of it. This review gives a comprehensive account of nanocellulose-water interactions and their repercussions in all key areas of contemporary research: fundamental physical chemistry, chemical modification of nanocellulose, materials applications, and analytical methods to map the water interactions and the effect of water on a nanocellulose matrix.

Original language	English
Pages (from-to)	1925-2015
Number of pages	91
Journal	Chemical Reviews
Volume	123
Issue number	5
Early online date	1 Feb 2023
DOIs	https://doi.org/10.1021/acs.chemrev.2c00611
Publication status	Published - 8 Mar 2023
MoE publication type	A2 Review article, Literature review, Systematic review

Funding

We acknowledge the community at the Department of Bioproducts and Biosystems at Aalto University for constructive discussions with numerous colleagues. K.H., W.X., and V.G. acknowledge the postdoctoral grants received from the Academy of Finland (grant numbers 333905, 349109, and 347219, respectively). This work is a part of FinnCERES Bioeconomy cluster, funded by the Academy of Finland.

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10.1021/acs.chemrev.2c00611Licence: CC BY

CHEM_Solhi_et_al_Understanding_Nanocellulose-Water_Interactions_2023_Chemical_ReviewsFinal published version, 54.5 MBLicence: CC BY

Cite this

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title = "Understanding Nanocellulose-Water Interactions: Turning a Detriment into an Asset",

abstract = "Modern technology has enabled the isolation of nanocellulose from plant-based fibers, and the current trend focuses on utilizing nanocellulose in a broad range of sustainable materials applications. Water is generally seen as a detrimental component when in contact with nanocellulose-based materials, just like it is harmful for traditional cellulosic materials such as paper or cardboard. However, water is an integral component in plants, and many applications of nanocellulose already accept the presence of water or make use of it. This review gives a comprehensive account of nanocellulose-water interactions and their repercussions in all key areas of contemporary research: fundamental physical chemistry, chemical modification of nanocellulose, materials applications, and analytical methods to map the water interactions and the effect of water on a nanocellulose matrix.",

author = "Laleh Solhi and Valentina Guccini and Katja Heise and Iina Solala and Elina Niinivaara and Wenyang Xu and Karl Mihhels and Marcel Kr{\"o}ger and Zhuojun Meng and Jakob Wohlert and Han Tao and Cranston, \{Emily D.\} and Eero Kontturi",

note = "Funding Information: We acknowledge the community at the Department of Bioproducts and Biosystems at Aalto University for constructive discussions with numerous colleagues. K.H., W.X., and V.G. acknowledge the postdoctoral grants received from the Academy of Finland (grant numbers 333905, 349109, and 347219, respectively). This work is a part of FinnCERES Bioeconomy cluster, funded by the Academy of Finland. Publisher Copyright: {\textcopyright} 2023 The Authors. Published by American Chemical Society.",

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month = mar,

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doi = "10.1021/acs.chemrev.2c00611",

language = "English",

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journal = "Chemical Reviews",

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T1 - Understanding Nanocellulose-Water Interactions: Turning a Detriment into an Asset

AU - Solhi, Laleh

AU - Guccini, Valentina

AU - Heise, Katja

AU - Solala, Iina

AU - Niinivaara, Elina

AU - Xu, Wenyang

AU - Mihhels, Karl

AU - Kröger, Marcel

AU - Meng, Zhuojun

AU - Wohlert, Jakob

AU - Tao, Han

AU - Cranston, Emily D.

AU - Kontturi, Eero

N1 - Funding Information: We acknowledge the community at the Department of Bioproducts and Biosystems at Aalto University for constructive discussions with numerous colleagues. K.H., W.X., and V.G. acknowledge the postdoctoral grants received from the Academy of Finland (grant numbers 333905, 349109, and 347219, respectively). This work is a part of FinnCERES Bioeconomy cluster, funded by the Academy of Finland. Publisher Copyright: © 2023 The Authors. Published by American Chemical Society.

PY - 2023/3/8

Y1 - 2023/3/8

N2 - Modern technology has enabled the isolation of nanocellulose from plant-based fibers, and the current trend focuses on utilizing nanocellulose in a broad range of sustainable materials applications. Water is generally seen as a detrimental component when in contact with nanocellulose-based materials, just like it is harmful for traditional cellulosic materials such as paper or cardboard. However, water is an integral component in plants, and many applications of nanocellulose already accept the presence of water or make use of it. This review gives a comprehensive account of nanocellulose-water interactions and their repercussions in all key areas of contemporary research: fundamental physical chemistry, chemical modification of nanocellulose, materials applications, and analytical methods to map the water interactions and the effect of water on a nanocellulose matrix.

AB - Modern technology has enabled the isolation of nanocellulose from plant-based fibers, and the current trend focuses on utilizing nanocellulose in a broad range of sustainable materials applications. Water is generally seen as a detrimental component when in contact with nanocellulose-based materials, just like it is harmful for traditional cellulosic materials such as paper or cardboard. However, water is an integral component in plants, and many applications of nanocellulose already accept the presence of water or make use of it. This review gives a comprehensive account of nanocellulose-water interactions and their repercussions in all key areas of contemporary research: fundamental physical chemistry, chemical modification of nanocellulose, materials applications, and analytical methods to map the water interactions and the effect of water on a nanocellulose matrix.

UR - https://www.scopus.com/pages/publications/85147442731

U2 - 10.1021/acs.chemrev.2c00611

DO - 10.1021/acs.chemrev.2c00611

M3 - Review Article

AN - SCOPUS:85147442731

SN - 0009-2665

VL - 123

SP - 1925

EP - 2015

JO - Chemical Reviews

JF - Chemical Reviews

IS - 5

ER -

Understanding Nanocellulose-Water Interactions: Turning a Detriment into an Asset

Abstract

Funding

Access to Document

Other files and links

Fingerprint

MimetiCell/Guccini: Biomimetic nanocellulose-based biohybrids with immobilized photosynthetic co-culture for wastewater remediation and carbon capture

-: FinnCERES

SYMBIOCELL: Symbiosis of surface-induced multicomponent reactions and Pickering emulsions as advanced synthetic tools for nanocellulose modification

Cite this

Understanding Nanocellulose-Water Interactions: Turning a Detriment into an Asset

Abstract

Funding

Access to Document

Other files and links

Fingerprint

Projects

MimetiCell/Guccini: Biomimetic nanocellulose-based biohybrids with immobilized photosynthetic co-culture for wastewater remediation and carbon capture

-: FinnCERES

SYMBIOCELL: Symbiosis of surface-induced multicomponent reactions and Pickering emulsions as advanced synthetic tools for nanocellulose modification

Cite this