Nanoscale thickness Octave-spanning coherent supercontinuum light generation

Susobhan Das, Md Gius Uddin, Diao Li, Yadong Wang, Yunyun Dai, Juha Toivonen, Hao Hong, Kaihui Liu, Zhipei Sun

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Abstract

Coherent broadband light generation has attracted massive attention due to its numerous applications ranging from metrology, sensing, and imaging to communication. In general, spectral broadening is realized via third-order and higher-order nonlinear optical processes (e.g., self-phase modulation, Raman transition, four-wave mixing, multiwave mixing), which are typically weak and thus require a long interaction length and the phase matching condition to enhance the efficient nonlinear light-matter interaction for broad-spectrum generation. Here, for the first time, we report octave-spanning coherent light generation at the nanometer scale enabled by a phase-matching-free frequency down-conversion process. Up to octave-spanning coherent light generation with a −40dB spectral width covering from ~565 to 1906 nm is demonstrated in discreate manner via difference-frequency generation, a second-order nonlinear process in gallium selenide and niobium oxide diiodide crystals at the 100-nanometer scale. Compared with conventional coherent broadband light sources based on bulk materials, our demonstration is ~5 orders of magnitude thinner and requires ~3 orders of magnitude lower excitation power. Our results open a new way to possibly create compact, versatile and integrated ultra-broadband light sources.
Original languageEnglish
JournalLIGHT: SCIENCE & APPLICATIONS
Volume14
Issue number1
DOIs
Publication statusPublished - 2025
MoE publication typeA1 Journal article-refereed

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