Improved operation of SO2 depolarized electrolyser stack for H2 production at ambient conditions

M. M. Gasik, J. Virtanen, A. Santasalo-Aarnio*

*Corresponding author for this work

Research output: Contribution to journalArticleScientificpeer-review

9 Citations (Scopus)
130 Downloads (Pure)

Abstract

In this paper, the performance of a robust SO2 depolarized electrolyser (SDE) stack that involves neither Pt catalyst nor carbon compounds at ambient conditions is demonstrated. In particular, the effect of different anolyte flow configurations to the overall H2 production rate and SO2 carry-over phenomenon is presented. These results indicate that serpentine anolyte flow (U-configuration) provides higher SO2 conversion, however, results in a more severe SO2 carry-over phenomenon due to increased membrane-electrolyte interface. In addition, individual unit cells in the stacks are monitored for further understanding about the different operational environment in each cell and to provide guidelines for future SDE stack design.

Original languageEnglish
Pages (from-to)13407-13414
JournalInternational Journal of Hydrogen Energy
Volume42
Issue number19
Early online dateMar 2017
DOIs
Publication statusPublished - 23 Mar 2017
MoE publication typeA1 Journal article-refereed

Keywords

  • Bipolar plates
  • Hydrogen production
  • Stack
  • Sulphur depolarised electrolyser

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