Energy absorption and resilience in quasi-static loading of foam-formed cellulose fibre materials

To avoid microplastic pollution, there is an urgent need to replace fossil-based cushioning materials in packaging with easily recyclable alternatives. Here, we investigated the potential of lightweight cellulose fibre materials as a solution for mechanical protection. The quasi-static compression was studied among a vast set of 129 different foam-formed trial points with material density ranging from 21 kg/m³ to 123 kg/m³. The trial points included two different fibre types, bleached softwood kraft pulp (BSKP) and bleached chemithermomechanical pulp (CTMP), with varied refining level, pulp consistency, foaming conditions, surfactant type, strength additives, and final material density and thickness. Besides a correlation analysis of factors affecting compression stress and resilience, the results were reflected against a new theoretical prediction of energy absorption for an ideal low-density random fibre network. The theory predicts the initially-high cushion factor to rapidly drop down to the level of 4‒5 at 40‒80% compression. A similar behaviour was seen among the actual samples, despite their various non-ideal features. At 50% compression, the average cushion factor across the whole data set was 4.84 ± 0.10, being close to the theoretical prediction of 4.61 for the ideal case. The smallest cushion factor of 3.6 was found for a CTMP sample. The recovery from compression varied slightly among the samples and appeared highest for the material density of 60‒100 kg/m³, following the predicted proportion of non-buckled fibre segments. According to the results, cellulose fibre-based cushions have a soft initial response, which is preferable for fragile items. Graphical abstract: (Figure presented.).