A comprehensive evaluation of crumb rubber modified asphalt-aggregate interfacial behavior and the effect of water : Molecular dynamics simulation and experimental investigation

Guojing Huang, Zixuan Chen*, Yanqiu Bi, Shuai Wang, Jiupeng Zhang, Augusto Cannone Falchetto

*Corresponding author for this work

Research output: Contribution to journalArticleScientificpeer-review

1 Citation (Scopus)

Abstract

The incorporation of crumb rubber (CR) makes the asphalt-aggregate interfacial properties highly complex and uncertain, while water is a key environmental factor causing interfacial failure. This paper aims to evaluate the characteristics of crumb rubber modified asphalt (CRMA)-aggregate interaction and the interfacial failure mechanism under the influence of different material properties and water at ambient temperature. Firstly, the CRMA-aggregate interfacial behavior before and after water intrusion is investigated using molecular dynamics simulations at the molecular scale. Next, the failure process and characteristics of the CRMA-aggregate interface were analyzed using the disk-shaped compact tension (DCT) test at the macro scale. Finally, the effect of water intrusion on the interface failure mode was analyzed through image processing. The results show that CR enhances binder cohesion and significantly affects its adhesion to aggregates with high CaO and MgO contents regardless of the presence of water. The asphalt concentration distribution on the CaO and MgO surfaces is more concentrated with higher peak concentration, leading to superior interfacial adhesion and water damage resistance with binder, while Al2O3 and SiO2 were inferior. The use of asphalt with higher creep stiffness, high-strength alkaline aggregates, and smaller CR particle size is beneficial for enhancing the CRMA binder-aggregate interfacial fracture performance. Water intrusion severely affected the interfacial adhesion, resulting in a significant increase in the proportion of adhesion failure, which is the main cause of the deterioration of the interface properties. The findings of this study provide insights into the factors affecting the CRMA-aggregate interfacial behavior, which facilitate the accurate design and application of high-strength durable CRMA mixtures.

Original languageEnglish
Article number132824
Number of pages14
JournalFuel
Volume377
DOIs
Publication statusPublished - 1 Dec 2024
MoE publication typeA1 Journal article-refereed

Keywords

  • Crumb rubber modified asphalt
  • Disk-shaped compact tension test
  • Interfacial behavior
  • Molecular dynamics simulation
  • Water

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